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I think you need to look much more to art direction and lighting to create that kind of look. Picture profile settings would be a part of getting your look but don't really mean anything apart from the actual shots. There's no "Amelie" look.
For the exteriors and available light scenes you really just have to play with it yourself.
Anyone knows how to get 'Amelie' look effect using picture profile settings? Some sort of warm greenish picture? Maybe someone tried?