Monochrome on camera or on post-production?

Yes, you can choose what colors should contribute to the blacks and whites. The look changes heavily if you lean it more to the blues or to the reds and so on.
 
Camera! :)

You have to be quite good to achieve the look and punch of the Nikon processing in post.
I like the B&W from the camera a lot especially with the Yellow filter turned on.
 
Normally i'd say post but with the heavy compression applied i'd do it in camera for a sharper and cleaner look. You can always manipulate the scale with filters, digital or optical.
 
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